Characteristics and corrosion protection of polypyrrole doped with salicylate anions on CT3 steel passivated by molydate
Email:
lanhtt@utc.edu.vn
Từ khóa:
Polypyrrole, corrosion protection, CT3 steel, sodium salicylate.
Tóm tắt
In recent years, the conducting polymers have attracted much attention in research and development because of their applications in medical and civil engineering. Here, the salicylate doped polypyrrole films were prepared on the carbon steel surface and their corrosion protection in 3 % NaCl solution were studied. Polypyrrole (Ppy) film was electrochemically synthesised with constant current techniques in a sodium salicylate solution (0.05M, 0.1M, 0.15M) and 0.1M pyrrole monomer on mild CT3 steel electrode passivated by molybdate. The morphological, structural, composition and thermal properties of salicylate doped Ppy films were characterized by scanning electron microscopy (SEM), Fourier transform infrared (FTIR) spectroscopy, and thermogravimetric analysis (TGA) techniques. The anti-corrosion ability of these films was assessed by electrochemical measurements in 3 % NaCl solution. The obtained results suggested that salicylate anions contributed in corrosion protection ability of Ppy films for mild steel electrode. The concentration of sodium salicylate of 0.1M and pyrrole of 0.1M is most suitable for preparation of good protection coating. The self-healing mechanism has been also mentioned for salicylate doped Ppy films on CT3 steel substrate.Tài liệu tham khảo
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[2]. K. Cysewska, S. Virtanen, P. Jasiński, Study of the electrochemical stability of polypyrrole coating on iron in sodium salicylate aqueous solution, Synthetic Metals, 221 (2016) 1-7. https://doi.org/10.1016/j.synthmet.2016.09.022
[3]. M. B. Gonzalez, L. I. Brugnoni, S. B. Saidman, Salicylate release from a polypyrrole matrix, Materials Today Communications, 18 (2019) 119–123. https://doi.org/10.1016/j.mtcomm.2018.11.012
[4]. A. C. Cascalheira, S. Aeiyach, P. C. Lacaze, L. M. Abrantes, Electrochemical synthesis and redox behaviour of polypyrrole coatings on copper in salicylate aqueous solution, Electrochimica Acta, 48 (2013) 2523-2529. https://doi.org/10.1016/S0013-4686(03)00295-0
[5]. S. Sirivisoot, R. Pareta, T.J. Webster, Electrically controlled drug release from nanostructured polypyrrole coated on titanium, Nanotechnology, 22 (2011) 085101.
https://doi.org/10.1088/0957-4484/22/8/085101
[6]. W. Prissanaroon-Ouajai, N. Koedsombat, N. Subbua, Novel Polyacrylamide/Polypyrrole Hydrogel for Electrically Controlled Release of Salicylic Acid, Key Engineering Materials, 824 (2019) 176–181. https://doi.org/10.4028/www.scientific.net/KEM.824.176
[7]. M. H. A. Zavar, S. Heydari, G. H. Rounaghi, Electrochemical Determination of Salicylic Acid at a New Biosensor Based on Polypyrrole-Banana Tissue Composite, Arabian Journal for Science and Engineering, 38 (2013) 29–36.
[8]. L. Wang, X. Li, Y. Yang, Preparation, properties and applications of polypyrroles, Materials Science. Reactive & Functional Polymers, 47 (2001) 125-129. https://doi.org/10.1016/S1381-5148(00)00079-1
[9]. T. V. Vernitskaya, O. N. Efimov, Polypyrrole: a conducting polymer; its synthesis, properties and applications, Russian Chemical Reviews, 66 (1997) 443.
[10]. P. M. George, A. W. Lyckman, D. A. LaVan, Fabrication and biocompatibility of polypyrrole implants suitable for neural prosthetics, Biomaterials, 26 (2005) 3511-3519. https://doi.org/10.1016/j.biomaterials.2004.09.037
[11]. H. Nguyen Thi Le, B. Garcia, C. Deslouis, Q. Le Xuan, Corrosion protection and conducting polymers: polypyrrole films on iron, Electrochimica Acta, 46 (2001) 4259-4272. https://doi.org/10.1016/S0013-4686(01)00699-5
[12]. F. Becka, R. Michaelis, B. Zinger, Filmforming electropolymerization of pyrrole on iron in aqueous oxalic acid, Electrochimica Acta, 39 (1994) 229–234. https://doi.org/10.1016/0013-4686(94)80058-8
[13]. Ha Manh Hung, Truong Thi Nga, Le Minh Duc, Tran Vinh Dieu, Vu Quoc Trung, Synthesis and properties of polypyrrole film by electrochemical method in citric acid on CT3 steel, Journal of Chemistry, 51 (2013) 277-281.
[14]. Vu Quoc Trung, Trinh Hong Hanh, Tran Hong Quang, Ha Manh Hung, Duong Khanh Linh, Hoang Thi Tuyet Lan, Le Minh Duc, Corrosion protection of molybdate doped polypyrrole film prepared in succinic acid solution, Corrosion engineering, Science and Technology, 53 (2018) 59–66. https://doi.org/10.1080/1478422X.2017.1389370
[15]. Zhihao Chen, Wenzhong Yang, Bin Xu, Yangyang Guo, Yun Chen, Xiaoshuang Yin, Ying Liu, Corrosion behaviors and physical properties of polypyrrole-molybdate coating electropolymerized on carbon steel, Progress in Organic Coatings, 122 (2018) 159-169. https://doi.org/10.1016/j.porgcoat.2018.05.022
[16]. Ha Manh Hung, Duong Khanh Linh, Nguyen Thuy Chinh, Le Minh Duc, Vu Quoc Trung, Improvement of the corrosion protection of polypyrrole coating for CT3 mild steel with 10-camphorsulfonic acid and molybdate as inhibitor dopants, Progress in Organic Coatings, 131 (2019) 407-416. https://doi.org/10.1016/j.porgcoat.2019.03.006
[17]. Andrea Santos Liu, Evelise Machado Ferri da Silva, Liu Yao Cho, The Chemical Deposition of Polypyrrole at a Copper Surface Varying Concentrations of Salicylic Acid in the Reactive Medium, Materials Science Forum, 1012 (2020) 447-452. https://doi.org/10.4028/www.scientific.net/MSF.1012.447
[18]. Dora M. Brasher, Role of the Anion in relation to Metallic Corrosion and Inhibition, Nature, 193 (1962) 868–869.
[19]. Natalya V.Likhanova, P.Arellanes-Lozada, O.Olivares-Xometl, H.Hernández-Cocoletzi, Irina V.Lijanova, Janette Arriola-Morales, J.E.Castellanos-Aguila, Effect of organic anions on ionic liquids as corrosion inhibitors of steel in sulfuric acid solution, Journal of Molecular Liquids, 279 (2019) 267-278. https://doi.org/10.1016/j.molliq.2019.01.126
[20]. Vu Quoc Trung, Pham Van Hoan, Duong Quang Phung, Le Minh Duc, Le Thi Thu Hang, Double corrosion protection mechanism of molybdate doped polypyrrole/montmorillonite nanocomposites, Journal of Experimental Nanoscience, 9 (2012) 282-292. https://doi.org/10.1080/17458080.2012.656710
[21]. Q. Pei, R. Qiuan, Electrode potentials of electronically conducting polymer polypyrrole Electrochimica Acta, 37 (1992) 1075-1081. https://doi.org/10.1016/0013-4686(92)85225-A
[22]. Le Minh Duc, Vu Quoc Trung, Layers of Inhibitor Anion–Doped Polypyrrole for Corrosion Protection of Mild Steel, DOI: 10.5772/54573, in book: Materials Science - Advanced Topics, Edited by Yitzhak Mastai, Intechopen Publisher, ISBN: 978-953-51-1140-5, 2013. https://www.intechopen.com/chapters/44936
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Kiểu trích dẫn
Hoang Thi Tuyet, L., & Lai Thi, H. (1631638800). Characteristics and corrosion protection of polypyrrole doped with salicylate anions on CT3 steel passivated by molydate
. Tạp Chí Khoa Học Giao Thông Vận Tải, 72(7), 789-799. https://doi.org/10.47869/tcsj.72.7.2
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